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Lane, Patricia M.
May 15, 2008
Suddenly on May 13, 2008, PATRICIA MARY LANE,
For the Orioles, the American League East is suddenly there for the taking
Peter Schmuck
August 9, 2014
Suddenly, it seems like it's all right there for the taking, and everyone - the Orioles, their fans and maybe even their closest competition - senses the leaves are going to turn orange and black in the fall. The Orioles moved to six games ahead in the American League East on Saturday with a resounding, 10-3 victory over the St. Louis Cardinals, in which they flexed their considerable muscles for the second day in a row before a national television audience. The Orioles now have the third-best record in baseball and the biggest lead of any of the six divisions.
Barda, Andy
August 12, 2007
Suddenly, on Monday, July 30, 2007, Andy Barda Funeral services will be held in Charlotte, NC.
One dead, eight injured by falling trees at Carroll County summer camp during storm
By Colin Campbell, The Baltimore Sun
July 8, 2014
One child was killed and eight others were injured by falling tree branches at a Christian summer camp in Carroll County during Tuesday night's storm, a fire department spokesman said. The children were on their way inside at River Valley Ranch in the 4400 block of Grave Run Rd. in Manchester around 7 p.m. when heavy winds brought branches from several trees down on top of them, said Donald Fair, public information officer for the Lineboro Volunteer Fire Department. Fair called the storm "very sudden" and said it caused "massive damage to the trees" in the area.
Parker, Nancy
December 29, 2008
Suddenly on December 27, 2008, Nancy Parker Interment private. Send condolences to www.ambrosefuneralhomes.com
Stevens, Louise W.
June 4, 2003
LOUISE WINIFRED STEVENS, died suddenly May, 28, 2003. Services at Garden of Faith Chapel at 12 P.M., June 6.
Good morning
March 2, 2006
Good morning --NFL players -- With so many of you suddenly about to be looking for jobs, have you thought of Monster.com?
Bozel, Jr, William
December 16, 2007
WILLIAM BOZEL, JR., born September 22, 1926 in Balitmore, MD, died suddenly November 27, 2007 in Cairo, GA. He was a proud career United States Marine. Private interment was held in Tallahassee, Florida on December 1, 2007.
Jefferson, Arnetha
June 7, 2006
ARNETHA JEFFERSON, passed away suddenly on June 1, 2006. Wife of Paul Jefferson. Mother of Malachi (Dusty) Jefferson, Stephanie Bannerman and Nacola Jefferson. There will be a memorial service held on June 9, 2006 at the Gospel Tabernacle Church, 206 Balnew Ave., Baltimore, MD from 4 to 6 P.M.
In Thursday's article on O. J. Simpson memorabilia, Jerry...
June 26, 1994
In Thursday's article on O. J. Simpson memorabilia, Jerry Warner of Mack the Plaque was quoted as being critical of some collectors. He was referring only to people who suddenly wanted Simpson items because of the notoriety of the murder charges against him.
John Tillman does not sound too concerned about Maryland men's lacrosse's sudden woes on offense
By Edward Lee and The Baltimore Sun
April 16, 2014
During a 7-0 opening stretch, Maryland averaged 13.1 goals per game. Since then, the Terps are 2-2 and have scored 10.5 goals per game - a number that would drop to 7.7 if a 19-6 thumping of Robert Morris on April 2 was left out of the equation. The sudden power outage is eerily similar to last year's progression, as that squad scored at least 10 goals in its first six games before failing to reach the double-digit mark in six of the last eight. But coach John Tillman did not sound alarmed about the offense's inability to find success against No. 7 North Carolina (eight goals in a three-goal loss)
Top city workers' compensation claim hit $624,000, Sun analysis shows
Scott Calvert, The Baltimore Sun
February 17, 2014
In October 2012, a Baltimore City firefighter was caught in a sudden burst of flames, suffering burns to his head, neck, shoulder, face and hand, according to a summary provided by the city. The firefighter has since won a workers' compensation award that the city anticipates will total $624,0000, making it the costliest claim filed by a city employee in the last fiscal year, records show. All told, the city expects to pay more than $35 million for 3,700 claims, with the bulk compensating for lost wages, medical bills and permanent physical injury.
Robert B. Reich: GOP's divide-and-conquer strategy no longer applies
By Robert B. Reich
January 15, 2014
Fifty years ago, when Lyndon Johnson declared war on poverty, the poor were different -- "other," as in Michael Harrington's seminal book of 1962, "The Other America. " That's no longer the case. After the War on Poverty ended, Republicans told working-class whites that their hard-earned tax dollars were being siphoned off to pay for "welfare queens" (as Ronald Reagan decorously dubbed a black single woman on welfare) and other nefarious loafers. The poor were "them" -- lazy, dependent on government handouts and overwhelmingly black -- in sharp contrast to "us," who were working ever harder, proudly independent (even sending wives and mothers to work in order to prop up family incomes dragged down by shrinking male paychecks)
As Tigers rise, 'all of a sudden, Towson is a destination for people'
Peter Schmuck
January 4, 2014
Even with the final seconds ticking away and the unhappy outcome of the Football Championship Subdivision championship game long since assured, there were no heads hanging among the Towson faithful gathered at Mother's Peninsula Grille in Arnold. The Tigers hit the ground running and, for a large chunk of the first half, seemed destined to embarrass the oddsmakers who had made them a huge underdog against the two-time defending FCS-champion Bison of North Dakota State. But their title hopes unraveled late in the second quarter, and the Bison three-peat came even easier than the double-digit point spread gave reason to expect.
Ravens' players and fans come to terms with sudden end to season
By Jeff Zrebiec, The Baltimore Sun
December 29, 2013
The final group of Ravens started trickling out of the visiting locker room at Paul Brown Stadium Sunday evening, heading first to Baltimore and then into an offseason that started far earlier than it expected. For the first time since 2007, the Ravens will be at home when the postseason begins, their season ending with a 34-17 loss to the Cincinnati Bengals. With their elimination, the Ravens become the fourth reigning Super Bowl champion in the past eight years to not make the playoffs the following season.
Ravens suddenly back in AFC playoff hunt, but still need to fix 'little things'
By Jeff Zrebiec, The Baltimore Sun
November 29, 2013
In a Ravens locker room flooded with a mixture of excitement, frustration and relief late Thursday night, running back Ray Rice sent a message to those who had already forecast his team's demise. "The Ravens are back," he said, swept up in the emotion of the team's biggest win all season. Their postseason hopes on life support less than two weeks ago, the Ravens woke up Friday in the AFC's sixth-and-final playoff slot. A pulsating 22-20 victory over the rival Pittsburgh Steelers on Thanksgiving night, secured when Emmanuel Sanders dropped a potential game-tying, two-point conversion with a little more than a minute to go, gets the Ravens back to the .500 mark at 6-6. Regardless of what happens Sunday with the AFC's four 5-6 teams, the Ravens will have possession of the sixth spot heading into their next game on Dec.8 against the Minnesota Vikings at M&T Bank Stadium, thanks to their 6-4 conference record.
Doneghy, Shirley E.
June 16, 2006
On June 1, 2006, SHIRLEY ELSIERDONEGHY, died suddenly of a heart attack after collapsing in her home. Surviving is a loving sister, Carole Doneghy of New York City. There will be a memorial service at Metropolitan UM Church, 1121 W. Lanvale Street, Monday, June 19, 6 P.M.
Talking to an earlier version of your father
By Clarence Page
May 14, 1996
WASHINGTON -- Your 6-year-old son has been playing quietly with Power Rangers and his other beloved action figures on the recreation-room carpet.Suddenly his face, a little peachy-cheeked replica of your own, looks up at you curiously.Then he slowly asks you a question that just sucks the breath right out of you.''Dad,'' he says, ''is Grandpa going to die?''A chain of questions races through your head: What does he know? How much has he heard? What should I say?So you answer his question with a question: ''Wh-Why do you ask?
Naval Academy employee dies suddenly
By Matthew Hay Brown, The Baltimore Sun
November 22, 2013
A civilian employee of the Naval Academy died Friday after falling unconscious on campus, the academy said. The woman, a member of the food service staff, was found unresponsive at about 5 a.m. in the kitchen area of King Hall, the academy said in a release. Another employee administered CPR until paramedics arrived, the academy said. The employee was taken to Anne Arundel Medical Center in Annapolis, where she was pronounced dead. The academy did not release the woman's name or any other details.
Port hits rough patch
October 19, 2013
At the beginning of the year, the Port of Baltimore was on a roll. At Seagirt Marine Terminal, the ribbon was cut on a 50-foot-deep berth financed by a $1.3 billion public-private partnership between the port and Ports America Chesapeake. The investment positioned Baltimore to be a major East Coast port of call for the larger ships expected in 2014 when the Panama Canal's expansion is completed. The port was doing record business: 9.55 million tons of cargo over the past fiscal year and a surge in the cruise business, too. The biggest concern was about how the port would find room to expand - and even that challenge looked like it would soon be met at Coke Point, the former iron ore pier at Sparrows Point, with plans to convert it into an automobile terminal and replace some of the 2,000 jobs lost when the steelmaking facility went out of business last year.
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subset: commoncrawl


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Floating hospital charts new seas
By William Cole
Advertiser Military Writer
By William Cole
PEARL HARBOR The USNS Mercy pulled into port yesterday following a four-month goodwill tour to the Pacific Rim that could signal a new mission for the hospital ship.
The Mercy's crew of military and civilian medical providers treated more than 60,000 people and performed more than 1,000 surgeries during port stops in the Philippines, Bangladesh, Indonesia and East Timor.
Among the onshore and on-ship locations where care was provided were Jolo, Zamboanga and Tawi-Tawi in the southern Philippines, where rebel activity makes humanitarian assistance difficult.
About 14 Philippines military personnel were killed in Tawi-Tawi the week before the medical team arrived in June, said Dr. Carl H. Lum, a surgeon from Hawai'i who volunteered for the mission.
And two weeks ago, an attack in Jolo killed about a half dozen other military members from the country, he said.
"We had high security alert and everywhere we went we were guarded by Filipino and American military troops," Lum said. "On land we wore flak jackets and steel helmets and we moved around only with convoys. We had Humvees in front of us, and Humvees in the back of us."
There were no attacks on the medical team, and it was able to treat a lot of people and perform surgeries on goiters and hernias and repair cleft lips and cataracts, Lum said.
"The surgery you do changes the life of the people completely," said Lum, who was with the Aloha Medical Mission. "If we weren't there, they wouldn't have the necessary surgery because none of the aid groups want to go there anymore because of security problems."
About 200 sailors, other military personnel and some of the up to 300 individuals with "non-governmental organizations," or NGOs, who took part in the humanitarian assistance mission were recognized yesterday by Adm. Gary Roughead, commander of U.S. Pacific Fleet, in a shipboard ceremony.
The organizations volunteering aboard Mercy included 32 individuals from Aloha Medical Mission, most of whom were from Hawai'i; Project HOPE; Operation Smile; Tzu Chi Foundation; International Relief Teams; the University of California at San Diego Pre-Dental Society and others.
"It was a voyage of teamwork and cooperation, but most importantly, it was a voyage of service and hope, and compassion brought together by so many, many people," Roughead said.
The medical team administered "tens of thousands" of shots and issued more than 60,000 pairs of eyeglasses, Roughead said.
The distinctively-marked converted supertanker, with its huge red crosses, stretches the length of three football fields and can accommodate up to 1,000 hospital beds.
The Mercy was delivered in 1986 and its sister ship, the Comfort, in 1987. The San Diego-based Mercy deployed to the Middle East for eight months in 1990 in support of the Gulf War.
After the December 2004 tsunami in Southeast Asia, Mercy was sent to the region for five months to provide humanitarian support and treated 107,000 patients in Indonesia, East Timor and Papua New Guinea.
The mission generated such positive feedback that officials decided to send the ship back this year without the urgency of disaster or war.
The Pentagon now prefers to airlift mobile combat hospitals into war zones instead of dispatching slow-moving hospital ships, the San Diego Union-Tribune reported. War casualties can be rapidly airlifted to receive advanced medical care in Germany and the United States.
Testifying this month before Congress on Islamic terrorism, Thomas M. Sanderson, deputy director of the Center for Strategic and International Studies, suggested building 10 hospital ships similar to Mercy to rebuild relations with Muslim countries.
"A lot of news is made of individual Iraqi children who are flown to the U.S. for special medical procedures, so imagine the impact of placing these hospital ships on rotation the world over," Sanderson said.
Capt. Joseph L. Moore, the commander of the medical treatment facility on Mercy, said higher echelons in the military will decide if Mercy makes a repeat humanitarian assistance trip to the region again next year.
"We're certainly hopeful that it will happen again," he said.
The medical equipment on the Mercy is state-of-art, Moore said.
Lum, who performed five major surgeries a day while the ship was in the Philippines, said "it's nice doing the surgery in a very up-to-date operating room. The operating rooms on the ship are as good as anywhere in the U.S."
Reach William Cole at email@example.com.


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With so many portable sound systems available for tablet and smartphone users, a product has to be extremely distinctive to really stand out. These Nunchuck Speakers metaphorically whack music listeners at first encounter, getting their attention with quite a novel design.
Inspired by the nunchuks of Japanese martial arts, this audio accessory comprises a pair of bluetooth-enabled amps that connect to each other by a flexible silicone cord. They can be wrapped around your iPad or your iPhone to perform the second function as a stand, and they can be easily carried around your neck or by hand to offer great portability. The 3Nod Group and Maxypro Nunchuck Speakers can also be fixed together into a closed loop for enhanced woofer quality.
Ninja Weapon Amplifiers
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- By: Amelia RoblinNov 14, 2013
References: red-dot.sg
References: red-dot.sg


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Home: Health: Eye Care
Bolle - Designer, manufacturer, and marketer of Bolle branded eyewear, including Bolle sunglasses, goggles, and tactical and safety eyewear.
EyecareInfo.com - Extensive and diverse Internet eye care information resource; information on optics, optometry and ophthalmology; eye care related news.
Lens Expressions - Secure online reseller of contact lenses and sunglasses at discount prices.
Home: Health: Eye Care


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Separate names with a comma.
Discussion in 'Apple Watch' started by FrisbeeK9, May 4, 2015.
Curious if anyone is looking their watch?
Yes. Silly not to. I set it to unlock with my iPhone so you basically never need to type it in and it protects your info should it get lost or stolen.
Yes. A passcode is required for Apple pay.
Absolutely. Just for peace of mind reasons alone.
That not the reason I will (and my wife does) lock it*. It's the same reason there's a lock code on the iPhone. Having someone look at my watch wasn't even a consideration originally.
(*thought the OP was saying to keep someone from "looking" at the watch display, but it's obviously a typo)
So, two reasons to lock the AW: First, it's an activation lock. Second, Apple Pay requires it (which makes sense).
Also, if you unlock your iPhone, it will unlock the Watch (we noticed a slight delay, but nothing that would affect actual use).
Oh is it? Didn't realize that. Thanks!


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How to Make Life Easier when Living with Mobility Issues
Mobility issues are something that no one should have to face. There is a daily toil that comes with…May 29, 2018
Mobility issues are something that no one should have to face. There is a daily toil that comes with…May 29, 2018
This may be a crazy concept, but your child may be able to build up immunity by playing in…March 12, 2018
As a parent, you do everything in your power to ensure your child is healthy and happy. However, did…November 17, 2017
In recent years the word "antioxidant" has been used ever more by marketing firms and in magazines, but what…October 20, 2017
The summer is approaching, which means that the most of your body will soon be exposed to the warm…April 4, 2017
If you want to lose weight as quickly as possible, the best possible way to go about doing so…March 15, 2017
Asthma is a common condition that can affect just about anyone, including children. As a parent, you'll no doubt…February 21, 2017
#AchievementForAll We've finally made it February and by this point, the resolutions have been abandoned or are starting to…February 2, 2017
Healthy habits are one of the most important things your kids need to learn from you. One UK study…October 3, 2016
Being a parent is one of the toughest jobs out there, and many feel that they are too overworked…September 6, 2016


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Going Deep Into Perfection With Group Structure Escape Room Games Tips Website Appeal OperationsFor your game info and guide website to be highly effective, you need to finish your research and think carefully about targeting your particular group. As soon as you know what kinds of men and women you must target, you can create your sales and promotions to fit their lifestyles, preferences, and demographics. Utilize specific key phrases throughout your website to provide a clear branding message. Look here to find techniques to develop a site designed to focus on your various market sectors.
Make the process of signing up easy, if it is a requirement of your game information and guide website. When you have your very own site, ensure that a registration procedure is a required needed step for consumers to acquire your product. Although some people will select not to sign up, it is typically a fantastic idea to give the alternative. Deals and special presents can attract consumers to sign up for an account, as well as recommendation benefit increases the variety of sign up.
The substance which you place on your video game information and guide site must match closely to your chosen keywords. If the keywords and the material do not align, you might draw the incorrect visitors to your site. The use of wrong keywords can harm the reputation of your site beyond repair. So, ask an expert designer to examine your website and provide a sincere critique, making sure you have actually chosen the very best words possible.
Could you escape from a gondola at 3,000m? Val Thorens challenges guests to do just that this spring
Inspired by the rising popularity of Escape Rooms, the concept that requires players to solve a series of clues in order to escape a themed scenario, Escape Game Caron takes place in the resort's 150-person Cime Caron cable car, which transports skiers and snowboarders to the Cime Caron summit at 3,200m. Could you escape from a gondola at 3,000m? Val Thorens challenges guests to do just that this spring
Hosting your video game information and guide site on an excellent server is necessary to run it successfully. Likewise, if you work with the top of the variety web-hosting company, you will have the ability to be sure that your website will never let you down. The success or failure of your site depends on the abilities of your webhosting. Do not hesitate to work with a brand-new webhosting if your website is failing to work correctly.
Ensure you have a video game details and guide site that any web browser is compatible with. The traffic to your online page can be optimized if every user is in a position to access the site with any device or browser. By not enabling the website to be accessible by all web browsers, you will sustain a great loss as many visitors will be limited from accessing the site. The person to make sure that your site runs efficiently on all web browsers is your web designer, so, remind him about it.
For you to increase your sales, you ought to embrace digital marketing together with sales promo at your physical place. Potential in-store consumers must understand that you exist for them to go to. By featuring your logo on business cards, print advertisements and letter head, you will strengthen your identity. Clients feel more safe when they realize that there is a private to listen to their worries when need emerge.


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Artist's description:
Three boatmen have tied up their boat on the Jumna (Yamuna) River shore by the Taj Mahal. It is a moonlit night, chilly enough to light a fire, the men sit around it eating a simple meal before going to sleep for an early start in the morning. Well that's how I see the story behind this picture, maybe you have your own?
This picture has a bit more Fantasy about it than most of my work although it is in keeping with recent trends in what I am painting.
Materials used:
oil on canvas
Featured by our Editors:
Moonlight Encampment (2014)
Oil painting by Mark Harrison
- Oil painting on Canvas
- One of a kind artwork
- Size: 15.75 x 11.81 x 0.79 in (unframed)
- Signed on the front
- Style: Illustrative
- Subject: Architecture and cityscapes
This artwork is sold by Mark Harrison from United Kingdom


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Shah Rukh Khan and Salman Khan
Bollywood superstar Shah Rukh Khan who unveiled the trailer of his upcoming film Zero on the occasion of his birthday on Friday said that he was touched by the gesture of Salman Khan doing a cameo in the film. During the trailer launch of the film when he was asked about how Salman came on board, Shah Rukh told the media: "Anand (L. Rai, Director) has spoken to Katrina (Kaif) regarding this film quite sometimes ago and that time Salman also heard the story.
"Then Salman called and said that there was this story and hear it. The coincidence is that, when finally, I said yes to the film, after that he said that I will be a part of this film for sure, by doing a song. That was very dignified and loving of him."
The film also features Anushka Sharma and Katrina Kaif. It is interesting to observe that after Yash Chopra's Jab Tak Hai Jaan this trio is coming together all over again to execute Rai's vision. Talking about her journey Anushka said: "This year I am completing 10 years in Bollywood. I made my debut with Shah Rukh and now after 10 years, in 2018 I am doing another film with him, it is so special and this is how life has come in a full circle."
In the film Shah Rukh is playing a character of a dwarf and Anushka and Katrina are playing a physically challenged person and an actress respectively. The film has slated to be released on December 21.
Also Read: From Karan Johar To Akshay Kumar, Celebs Praise Shah Rukh Khan's Zero Trailer
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Advances in Condensed Matter Physics
Volume 2015, Article ID 537860, 4 pages
Photoelectrochemical CO2 Conversion to Hydrocarbons Using an AlGaN/GaN-Si Tandem Photoelectrode
1Advanced Research Division, Panasonic Corporation, Seika, Kyoto 619-0237, Japan
2Department of Applied Physics, Tokyo University of Science, Katsushika, Tokyo 125-8585, Japan
Received 22 September 2014; Accepted 22 November 2014
Academic Editor: Junichiro Kono
Copyright © 2015 Masahiro Deguchi et al. This is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
We report on a qualitatively improved photoelectrochemical CO2 reduction system which makes it possible to convert CO2 into hydrocarbons. The key is the tandem photoelectrode, which consists of AlGaN/GaN and Si device with p-n junction. The Si device is located on the back of AlGaN/GaN structure and acts as activation layer that raises cathode potential. Use of a Cu cathode results in change of the main reaction products from CO and HCOOH to hydrocarbons such as CH4 and C2H4. The energy conversion efficiency to hydrocarbons from CO2 is estimated to be 0.046% under irradiation with concentrated solar light.
1. Introduction
The consumption of fossil fuels, which has been increasing exponentially since the early 20th century, is resulting in a rising concentration of carbon dioxide (CO2) in the atmosphere and is raising the risk of an economic crisis striking when conventional energy sources run out. To solve these two problems, there has been a great deal of research into how to reduce CO2 emissions, such as by energy-saving or carbon capture and storage. However, no matter by how much CO2 emissions can be reduced, the problem of eventual depletion of fossil fuels remains. At present, despite intensive efforts, it is still not possible to produce enough renewable energy to support human activities.
Photocatalytic energy conversion is one of the most intensively researched fields for producing renewable energy. Since photocatalytic water splitting was discovered, numerous photocatalysts have been synthesized for hydrogen production [1–5]. In photocatalytic reactions, the key is to design the band-gap structure of the photocatalyst to deliver the reaction energies needed for water splitting.
Another important photocatalytic reaction is CO2 reduction: it would enable us to reduce CO2 and produce carbon-based fuels simultaneously and thus would be a major step towards reducing and recycling CO2. However, a higher cathode energy is necessary for CO2 reduction than for H2O reduction, and it also involves water oxidation as a counterreaction. Because of the challenging nature of the process, there are far fewer research reports on this subject than those on hydrogen generation [6–11].
The authors have reported that the problem of high cathode potential required for CO2 reduction can be solved by using gallium nitride (GaN) as a photoelectrode [12, 13]. GaN is one of the few materials that can create excited electron-hole pairs with sufficient energy for CO2 reduction and water oxidation, which means it can be operated with no extra bias input or need for sacrificial materials. Recent research has established that the efficiency of the GaN photoelectrode can be considerably enhanced by creating an AlGaN/GaN heterostructure in which the main reaction product is formic acid (HCOOH) [14, 15].
Although HCOOH could be used as a renewable energy source, ideally CO2 should be converted to conventional fuels, such as hydrocarbons and alcohols. There are two requirements for realizing a conversion from CO2 to hydrocarbons. One is to raise the cathode potential sufficiently to promote a reaction with multiple electrons and protons, which is necessary for converting CO2 to methane. The other is to adopt a cathode catalyst that is able to drive such a complicated reaction.
For this purpose, to raise the cathode potential, we adopted a tandem structure comprising a photoelectrode with multilayered nitride semiconductors and a Si p-n junction. The Si p-n junction has the role of increasing the cathode potential via the photovoltaic effect. The increased cathode potential achieved by adopting a copper (Cu) electrode as the cathode also creates a qualitative difference. Cu is a CO2 conversion catalyst whose reaction products vary considerably according to the cathode potential [16, 17]. We succeeded in changing the main reaction products from carbon monoxide (CO) and HCOOH to hydrocarbons such as methane (CH4) and ethylene (C2H4).
2. Materials and Methods
The photoelectrode presented in this study consists of a tandem structure comprising an AlGaN/GaN region and Si with p-n junction as shown in Figure 1. The AlGaN/GaN region was unintentionally doped (uid-) AlGaN and highly Si-doped n+-GaN thin film layers grown epitaxially on a conductive GaN substrate: the same structure as described in our previous study [15]. It should be noted that the present study employs a GaN substrate to realize a vertical device with an Si p-n junction. The uid-AlGaN layer plays a role in the efficient conversion of photons to electron-hole pairs that are needed to trigger chemical reactions. This heterostructure appears to show electric polarization in the uid-AlGaN layer, which makes electron-hole separation more effective [14]. NiO co-catalysts are also supported on the GaN in the same manner as described in a previous report [18].
The Si with p-n junction described in Figure 1 is constructed by applying amorphous Si films to an n-Si single-crystal substrate that converts energy from light to electricity. The Si with p-n junction utilizes the light transmitted from the AlGaN/GaN region. The role of Si with p-n junction is to raise the cathode potential using the photovoltaic effect. The cyclic voltammetry measurements of the cathode suggest that the cathodic current should increase when the cathode potential is raised.
Two 300 W xenon arc lamps (Asahi Spectra) with spectroscopic mirrors were focused through quartz optical fibers onto the surface of the photoelectrode. The irradiation area was 9 cm2. Each lamp was fitted with UV- and VIS-mirrors and the power was appropriately tuned to imitate that of the real sun. The spectrum of the light used in the present study is shown in Figure 2 together with the spectrum of AM 1.5 (1-SUN, 100 mW/cm2) for comparison. Although wavelengths over 800 nm are attenuated due to the VIS-mirror, in this paper we define this spectrum as 1-SUN. The efficiency calculated in the latter discussion is based on measurements under the light spectrum described in this Figure 2.
The reaction products of CO2 conversion include liquid components, such as formic acid and alcohols. To completely prevent these liquid components from following inverse reactions, we used an H-type reactor to separate the cathode and anode by means of a cation exchange membrane (Dupont Nafion 117) that blocks electrolytic intercommunication. The electrons, excited by light illumination on the photoelectrode, move to the cathode where they drive the CO2 reduction reactions. Here, a Cu plate (Nilaco, 99.9999%) was chosen as the cathode for CO2 reduction, while the photoelectrode was placed at the anode.
The Cu electrode was immersed in 1.0 or 3.0 M KCl electrolyte on the cathode side, and the uid-AlGaN/n+-GaN photoelectrode was immersed in 5.0 M NaOH electrolyte on the anode side. Each electrolyte was selected so as to promote the reactions on each electrode. The photoelectrode is a 2-inch circular device while the surface area of the cathode metal is an 0.8 inch-diameter circle. The cathode and anode were electrically connected via an ammeter.
The cell for the cathode was hermitically sealed, and CO2 was introduced into the electrolyte by gas bubbling before photoelectrolysis. After the photoelectrochemical reduction, the gas and liquid samples were analyzed using gas and liquid chromatography, respectively. Hydrogen (H2) was determined using a thermal conductivity detector (TCD); and CO, CH4, C2H4, and ethane (C2H6) were determined using a flame ionization detector (FID) attached to a gas chromatograph (GL Sciences GC-4000). Liquid chromatography was used for detecting HCOOH (Shimadzu LC-2010). Alcohol components such as C2H5OH were detected by gas chromatography (Shimadzu GC-17A) connected by a headspace sampler (PerkinElmer Turbomatrix HS40).
3. Results and Discussions
We show the change in the reaction products in the photoelectrochemical CO2 reduction in Figure 3, with the Si with p-n junction adopted. This result was obtained under 3.0 M KCl electrolyte and 8 × 1-SUN (8-SUN). The production of hydrocarbons (CH4, C2H4) and alcohol (C2H5OH) was confirmed after adopting the Si p-n junction, whereas they appeared only in minute quantities in the previous study. The difference in the distribution of reaction products was consistent with the change in the cathode potential from –1.47 V versus Ag/AgCl to –1.74 V versus Ag/AgCl.
The energy conversion efficiency was estimated to be 0.034% under concentrated sunlight and reached 0.046% in case of 1.0 M KCl electrolyte. Here, the denominator for the estimation is 800 mW/cm2 (8-SUN) and the numerator is the sum of energies for hydrocarbons (CH4 and C2H4). As discussed above, the energy of the light we used is lower than real sunlight, especially at over 800 nm, which means that it is unlikely to be an overestimate.
This result also confirms that concentrated sunlight effectively raises the cathode potential. To realize hydrocarbon production under real sunlight, we constructed a photoelectrochemical CO2 conversion system with a lens and a tracking system for concentrating the sunlight. A picture of the system is shown in Figure 4(a). A 30 cm-square Fresnel lens is set in front of the photochemical cell. The measurement was carried out in July in Kyoto, Japan. The photocurrent between anode and cathode was measured during the experiment and is shown in Figure 4(b). On the day, the reaction was often interrupted by passing clouds; however, sufficient photocurrent was observed through measurement of the accumulated electric charges in the system. After 4 hours of photoelectrolysis, the accumulated electric charge was 104 C, and the measurements made using the gas chromatograph showed 285.3 ppm of methane and 251.8 ppm of ethylene, showing that approximately 0.74 μmol of hydrocarbons were generated from CO2 using real sunlight.
4. Conclusions
We have shown that Si with p-n junction brings about not only a quantitative but also a qualitative improvement in the CO2 photoelectrochemical system. The idea of using a p-n junction as the back surface of a photoelectrode has been discussed in several reports on hydrogen generation [19, 20]. Those results show its outstanding efficiency for producing hydrogen. In the system presented here, although the efficiency may not be outstanding, it brought a qualitative improvement in that the main reaction products changed from CO and HCOOH to hydrocarbons. The performance of the CO2 photoelectrochemical system is determined by the balance of several factors which are the properties of the cathode and anode, the electrode size, and light intensity. Further improvements will be accomplished by optimizing the properties of each factor.
Conflict of Interests
The authors declare that there is no conflict of interests regarding the publication of this paper.
The authors would like to thank Dr. M. Taguchi and S. Shimada for providing the Si device with p-n junctions and for fruitful discussions.
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Makers ensuring full comfort for pregnant Gurdeep Punj on 'Dil Ki Baatein Dil Hi Jaane' setsNew Delhi: Gurdeep Punj who will be seen in the latest Ram Kapoor starrer TV show 'Dil Ki Baatein Dil Hi Jaane' might have to flare a great courage while shooting for the show.
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Andrea Toto
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The poll is up!
Hi, I'm new here. Is this slog just a community reading of TDTCB at an established pace with thoughts/comments posted along the way? I'd like to participate, but not exactly sure what it is.
Quote from: Redeagl on February 10, 2017, 10:01:07 pmThe poll is up!I'm quite fond of PoN, TDTCB specifically. So, I'm good either way is chosen.