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Fan Guo,
Jin-Han Guo,
Peng Wang,
Yan-Shang Kang,
Yi Liu,
Jing Zhao* and
Wei-Yin Sun*
Coordination Chemistry Institute, State Key Laboratory of Coordination Chemistry, School of Chemistry and Chemical Engineering, Nanjing National Laboratory of Microstructures, Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210023, China. E-mail: firstname.lastname@example.com; email@example.com; Tel: +86 25 89683485
First published on 1st April 2019
Facet-dependent catalytic activity of hard materials such as metals and metal oxides is well recognized in previous works. However, it has rarely been established for metal–organic frameworks (MOFs), possibly because the soft crystals of MOFs are conceptually different from the hard solids. In this work, the surface structure of the MOF NH2-MIL-125(Ti) has been investigated by density functional theory (DFT) calculations for the first time. These calculations predict that the {110} facet has a surface energy of 1.18 J m−2, which is superior to those of the {001}, {100} and {111} facets. This difference can be attributed to the larger percentage of exposed metal clusters, which can act as active sites in catalysis. Thus, we have devised and successfully obtained a series of nanoscaled NH2-MIL-125(Ti) MOFs with controlled facets both experimentally and theoretically. The sample containing the {110} facet exhibits the highest photocatalytic hydrogen production activity and apparent quantum yield, which are approximately three times those of the sample with a dominant {111} facet.
In the case of titanium-based MOFs, NH2-MIL-125(Ti), one of the most thoroughly investigated MOF systems, has been revealed to have several semiconductor behaviours, including electron transfer from the photo-excited organic linkers to the metal-oxo clusters.25 Due to the efficiency and universality of catalytic processes, researchers have been inspired to explore NH2-MIL-125(Ti) and have already used this material for optical response,26 photocatalytic CO2 reduction,27 and oxidation of amines to imines.28 In these cases, the morphology of NH2-MIL-125(Ti) is one-fold, indicating its preference for the increased stability of the less reactive facet. Importantly, the growth of a MOF crystal surface is through a two-dimensional surface nucleation or a "birth and spread" growth mechanism. The height of each additional layer is that of a cluster or ligand.29 Jiang and Zheng et al. reported that the metal clusters played a significant role acting as active sites for the photocatalytic activity of catalysts.30,31 As a consequence, when a larger proportion of metal clusters exists on one surface, the facet possesses a higher activity and surface energy.
In this paper, the surface energies of different facets of NH2-MIL-125(Ti) were examined by density functional theory (DFT) calculations. The DFT theoretical calculations predict that the surface energy of the {110} facet is as high as 1.18 J m−2, and more clusters are exposed on that surface than on the {001}, {100} and {111} facets. We designed and accomplished a facile approach for the synthesis of nanoscaled NH2-MIL-125(Ti) with controlled facets and successfully incorporated the more reactive {110} facet. Electrochemical and photochemical measurements as well as control experiments have been carried out. The truncated tetragonal-like plates containing the {110} facet exhibit notable photoelectric correlation performance and the highest photocatalytic hydrogen generation activity, which is three times greater than that of octahedrons with dominant {111} facets. The apparent quantum yield (AQY) at 420 nm is as high as 3.60%. This is the first attempt to investigate the nature of photocatalytic activities from different facets of MOF materials by combining theoretical and experimental methods.
|Fig. 1 The creation of as-cut planes for the facets (a) {001}, (b) {110}, (c) {100} and (d) {111} by different coloured lines.
Inspired by the theoretical results, we set out to design and synthesize a series of NH2-MIL-125(Ti) crystals with different facets by varying the concentration of the structure-capping surfactant cetyltrimethylammonium bromide (CTAB) in a DMF–CH3OH solution. Scanning electron microscopy (SEM), enlarged SEM, transmission electron microscopy (TEM) images and the corresponding 3D geometric models shown in Fig. 2 revealed that different morphologies of NH2-MIL-125(Ti) were generated depending upon the amount of CTAB used. In the absence of the surfactant CTAB, the products are disk-like plates with two {001} facets, and the average diameter and thickness are estimated as 800 and 200 nm, respectively (Fig. 2a). Under the same reaction conditions, with the addition of 1 mM CTAB, facets of {001} still remained, but the morphology was changed to rounded rectangle-like plates (Fig. 2b). After increasing the concentration of CTAB to 2 mM, the appearance of eight {110} and eight {111} facets was noted, as shown in Fig. 2c. The morphology was changed to truncated tetragon-like plates, the mean particle size is approx. 600 nm, and the thickness remains at 200 nm. The angle of 77.36° in the equilateral triangle between two adjacent rectangles (Fig. 2c-enlarged SEM image) corresponds to the obtuse angle in the {110} facet between two {111} facets (Fig. 2c, 3D geometry model). Fig. 2d shows that the morphology of the sample has evolved into truncated octahedrons consisting of two {001}, four {100}, and eight {111} facets. The mean particle size, however, was maintained at approximately 600 nm when the concentration of CTAB was increased to 3 mM. The {110} facet disappeared because facets with a high surface energy tend to diminish rapidly during the crystal growth process so as to minimize the total crystal energy.8 When the concentration of CTAB was further increased to 4 mM, other facets disappeared, and octahedral nanoparticles with only {111} facets were obtained (Fig. 2e). The results demonstrate that by increasing the concentration of CTAB, an evolution of the nanoscaled NH2-MIL-125(Ti) morphology was observed, from disk-like plates, to rounded rectangle-like plates, to truncated tetragonal-like plates, to truncated octahedrons and finally to octahedrons. These samples are denoted as T001-1, T001-2, T110, T100, and T111, respectively, where T represents Ti, and 001/110/100/111 are the dominant facets. According to the SEM images in Fig. 2c–e, the average percentages of different facets are calculated for samples T110, T100, and T111 from the surface area of each facet and are given in Table S1.†32 SEM energy-dispersive spectra (SEM-EDS) elemental mapping images of the samples ensure the spatial distribution of Ti (Fig. S3†).
|Fig. 2 SEM, enlarged SEM, TEM images and the corresponding 3D geometry models of as-synthesized NH2-MIL-125(Ti) obtained under different concentrations of CTAB: (a) 0, (b) 1 mM, (c) 2 mM, (d) 3 mM and (e) 4 mM.
Powder X-ray diffraction (PXRD) data for the products are in good agreement with the simulated MIL-125(Ti), indicating that the framework structures are not influenced by the use of H2bdc-NH2 as an organic linker (Fig. S4†). It is noteworthy that the diffraction intensity ratio for the {110} and {220} facets in the PXRD pattern of sample T110 is obviously higher than those of the others, suggesting that the T110 has a greater possibility of exposing the {110} facet. Likewise, T001-1 and T111 generate the highest diffraction intensity ratio for the {002} and {222}, respectively. Therefore, the surfaces of T001-1 and T111 are dominated by {001} and {111} facets, severally.33 The results imply that the samples exhibit facet-dependent PXRD patterns, which is consistent with the crystal shapes observed by SEM results. Fourier transform infrared (FT-IR) spectra of NH2-MIL-125(Ti) samples have similar characteristic bands, and no cetyltrimethyl groups were detected (Fig. S5†). Similarly, X-ray photoelectron spectroscopy (XPS) data gave no signal for Br− (Fig. S6†), confirming that the samples are surfactant-free. In addition, the atomic concentrations of the samples examined by XPS, which is widely accepted as a surface analysis-based technique, are listed in Table S2.† The Ti 2p concentration of T110 is higher than other samples, indicating that there are more metal clusters on the outer surface of T110 than others. Thermogravimetric (TG) curves show the thermal stability of the samples (Fig. S7†). To ensure the porous structure of the as-synthesized NH2-MIL-125(Ti), N2 adsorption isotherms were measured at 77 K (Fig. S8†). Characteristic type-I sorption isotherms indicate that the samples are microporous materials with high amounts of N2 adsorption. The increase at pressures P/P0 = 0.9–1.0 might be attributed to the inter-particle adsorption that occurs in nanoscaled MOFs.34 The Brunauer–Emmett–Teller (BET) surface areas of these samples were calculated from the N2 adsorption isotherms (Fig. S8†). The results show that the samples exhibit morphology (facet)-dependent sorption properties. In addition, CO2 adsorption data were measured at 273 K (Fig. S9†), and a comparison of the CO2 adsorption with other amine-functionalized MOFs is provided in Table S3.†
To investigate the optical responses of the above samples, corresponding measurements were examined. UV-visible diffuse reflectance spectra show that all samples had a shift of light absorption from the UV to the visible region (Fig. 3a). Photoluminescence (PL) spectra for the products were measured under excitation at 326 nm (Fig. 3b). The steady-state PL spectra show that the PL band centred at approx. 420 nm is strong for T001-1 and T111, while it becomes weak for T001-2 and T100, and it is the weakest for T110. The evident PL quenching indicates that the most rapid and efficient electron transfer is in T110 among the above samples. Moreover, the photoresponsive properties were measured by the photocurrent–time curves, and all of the samples exhibit a clear photocurrent response under visible light irradiation (λ > 400 nm) at a pulse of 40 s (Fig. 3c). T110 in particular was found to have better photoresponse capability and interface charge separation efficiency than other samples. In addition, these results are also supported by electrochemical impedance spectroscopy (EIS). Fig. 3d shows that the capacitance arc for T110 is the smallest, indicating that it has the lowest charge-transfer resistance. It is well established that the different optical and electrochemical properties among the samples suggest their difference in driving the photocatalytic process.
|Fig. 3 (a) UV-visible diffuse reflectance spectra, (b) PL emission spectra, (c) photocurrent responses, and (d) EIS Nyquist plots for NH2-MIL-125(Ti) with different morphologies.
To assess the photocatalytic ability of NH2-MIL-125(Ti) nanomaterials for visible-light-driven hydrogen evolution, photocatalyst T001-1, T001-2, T110, T100 or T111 was added to a Pyrex reaction vessel containing a mixture of CH3CN and deionized water with triethanolamine (TEOA) as a sacrificial electron donor, and it was exposed to visible-light illumination. Fig. 4a shows the hydrogen evolution rates of photocatalytic hydrogen production under visible light irradiation for each of the five samples. T111 is able to generate a minimal amount of hydrogen, while the T001-1 and T001-2 samples give higher hydrogen production than T111 under identical conditions. Among these varied morphologies, the T110 sample displays the highest hydrogen production rate (60.8 μmol g−1 h−1), which is more than three times that of the T111 sample. More importantly, T110 exhibits almost constant activity even after 30 h during the recycling experiments for up to three cycles, demonstrating its high recyclability and stability for visible-light-driven hydrogen production (Fig. 4b). The SEM image (Fig. S10†) and PXRD pattern of T110 (Fig. S11†) after three catalytic recycles confirmed that the sample maintains its structure, suggesting its high stability under the photocatalytic conditions. Ligand-to-metal charge transfer occurs in NH2-MIL-125(Ti) with T110 as a photocatalyst, and this was confirmed by electron paramagnetic resonance (EPR) spectra (Fig. S12†).35,36 To examine the origin of the hydrogen, D2O was used in the photocatalytic reaction with the other experimental conditions remaining unchanged. The mass spectrometry data show that the resulting gas is a mixture of D2, HD and H2 (Fig. S13†), implying that the origin of hydrogen is from H2O and that the exchange of H+ between H2O and TEOA in the solution may occur. The time-dependence of the rates of hydrogen evolution of the photocatalysts is shown in Fig. S14,† and the hydrogen evolution rates with the previously reported NH2-MIL-125(Ti) and other MOF-based photocatalysts are summarized in Table S4.† It is clear that nanoscaled NH2-MIL-125(Ti) MOFs with definite facets lead to significantly enhanced photocatalytic activity compared to the reported NH2-MIL-125(Ti) materials and even to some MOF-based noble metal-hybrid photocatalysts. To better clarify the photocatalytic performance, the AQY for the hydrogen production37,38 of T110 was calculated to be 3.60% at 420 nm, while the AQY values of other samples including T001-1, T001-2, T100, and T111 are approximately 2.40%, 2.88%, 3.12%, and 1.44%, respectively. An AQY of 3.60% is higher than those of some inorganic semiconductors and correlative composites (Table S5†). The combination of theoretical simulations and experimental investigations suggested that the vital factor for the higher photocatalytic performance of T110 is the superior surface properties of the {110} facet.
|Fig. 4 (a) Photocatalytic hydrogen production using NH2-MIL-125(Ti) with different morphologies. (b) Recycling tests using T110.
|† Electronic supplementary information (ESI) available: XPS spectra, TG, PXRD, N2 adsorption and desorption isotherms, CO2 adsorption, SEM, EPR spectra, hydrogen production rate, surface structures, creating as-cut surfaces, and average percentages of different facets. Comparison tables regarding the CO2 adsorption, photocatalytic hydrogen production performances, and AQY of this work with other MOF photocatalysts reported in the literature. See DOI: 10.1039/c8sc05060k
|This journal is © The Royal Society of Chemistry 2019


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Rangers 2-1 Ayr United: Bilel Mohsni nets double as Ally McCoist's men close in on unbeaten Scottish League One season
So that's 34 down, two to go. In a campaign long since reduced to a numbers chase for a Rangers team bereft of genuine divisional competition, the figures continue to be amassed in their favour. If some of the performances don't bear too much in the way of close inspection, well, that's hardly their most pressing concern at the moment.
This gritty victory over an attractive Ayr United side was the 32nd league win of the season for Ally McCoist's men, who now stand just two shy of the 100-point mark – and within two closing games of completing their SPFL fixture list undefeated.
As McCoist himself acknowledges, there will be keen debate about where to rank the achievement of cutting an invincible swathe through the third tier of Scottish football. Arguments for another day.
Up and above: Rangers defender Bilel Mohsni rises highest in the box to score his side's opening goal
Rangers: Bell, Foster, Smith, Peralta Sosa (Clark 72), McCulloch, Mohsni, Aird, Black, Daly, Shiels (Gallagher 72), Law (Hutton 86)
Subs not used: Faure, Simonsen, Crawford, Telfer
Goals: Mohsni 54, 82
Ayr United: Hutton, McGowan, Pope, McLaughlin, Campbell, Lithgow, Forrest, Gilmour, Malcolm, Moffat, Donald
Subs not used: Kyle, Shankland, Crawford, Hunter, Marenghi, Longridge, Newman
Goal: Forrest 69
Bookings: Malcolm, Donald
Referee: Iain Brines
Attendance: 40,651
On Tuesday night at Ibrox, a Bilel Mohsni double either side of a super finish by Alan Forrest – the 17-year-old kid brother of Celtic star James – was enough to see off visitors who more than held their own for long enough.
United still harbour ambitions to join Rangers in the Championship, via the play-offs, and they look as if they'd be a decent addition to the league. They certainly made life more than difficult for a home side in pursuit of something more than just a title to show for their efforts.
Each step towards the inevitable has been its own little drama for Rangers, of course. Some more diverting than others.
On a cold and intermittently rain-spattered night, with top-class European football on council telly providing a counter-attraction, it must have been tough for even the most devoted of diehards to get motivated for this latest attempt at statistical perfection.
There would arguably have been as much pre-match interest in chief executive Graham Wallace's slightly underplayed revelation – near the very end of his programme notes – that the much-vaunted 120-day review of club finances had been completed. Not that he was giving anything away last night.
Two good: Mohsni celebrates as he scores a double in Rangers' 2-1 victory over Ayr United at Ibrox
Much depends on exactly what Wallace does or doesn't reveal in his 'update' later this week, of course. Credit the match-night announcer, then, for keeping the incredulity out of his voice as he plugged season-ticket renewals before kick-off; surely even his script writer must be aware of the, erm, debate regarding this very subject?
Out on the pitch, Rangers began this match in diligent if hardly spectacular fashion, sending in plenty of crosses, to which there were an equal number of Ayr United clearances. A zero sum equation may have a certain beauty to mathematicians – but it doesn't make for great entertainment.
The visitors actually put together the most threatening early move, Craig Malcolm curling a right-footed shot just wide of the far post after some sweet build-up play with strike partner Michael Moffat.
Rangers responded in their own time, Jon Daly sending a shot over after a cheeky Fraser Aird back-heel, before Arnold Peralta had a goal-bound effort brilliantly blocked by Ayr keeper David Hutton.
Close range: Mohsni scores Rangers' second goal just eight minutes from time
In the stands: Rangers chief executive Graham Wallace (right) and directors Sandy (centre) and James Easdale (left) applaud as they watch the action in Glasgow
There might well have been a feeling among home fans that their team would, sooner or later, find their way past decent but limited part-time opponents, if only through superior fitness eventually beginning to tell. Without naming names, one or two of the Ayr players looked on the hefty side of chunky.
In Malcolm and Moffat, though, they possess a strike pairing of no little prowess. When Michael McDonald forced Cammy Bell to dive at his feet to make a sharp save, we were reminded that United carried more than a fleeting threat.
The sight of Mohsni getting involved in an unnecessary row – over a throw-in at half-way, of all things – with Ayr boss Mark Roberts provided some diversion for fans beginning to grow weary of the pattern of play, as both teams created and wasted chances. Lee McCulloch and Moffat then both blazed efforts over the bar before half-time.
Touchline praise: McCoist congratulates Mohsni as his side edge closer to an unbeaten league season
Aird began the second half in lively style, getting at the right side of the Ayr defence with verve and pace. And the winger was involved, albeit in a more stationary manner, in the opener.
His corner from the left was hit with pace and dip, giving Mohsni the perfect opportunity to connect with a forceful downward header, giving Hutton no chance of making a save.
The central defender's 11th of the season had an obvious settling effect on Rangers, who began to pepper the Ayr goal with efforts. None good enough to beat Hutton, though.
Equaliser: Ayr United's Alan Forrest celebrates after pulling his side level in the 69th minute
They were made to pay for their profligacy when the hapless Peralta gifted possession to Scott McLaughlin just ouside the Rangers box, the midfielder beautifully picking out Forrest – whose super-cool finish bore all the hallmarks of a fine footballing pedigree.
The pressure was now on Rangers to rally. Step forward Mohsni, in the right place at the right time – 10 minutes from the end - to finish from close range after a Daly header had been blocked on the line.
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Load your family into the 2019 Mazda CX-5. Under the hood you'll find a 4 cylinder engine with more than 170 horsepower, and all wheel drive keeps this model firmly attached to the road surface. Top features include rain sensing wipers, a power seat, an automatic dimming rear-view mirror, front bucket seats, power moon roof, a power rear cargo door, blind spot sensor, and a split folding rear seat. Features such as automatic climate control and leather upholstery prove that economical transportation does not need to be sparsely equipped. Rear passengers enjoy the seat heating functionality, keeping them warm during the winter months. The unique heads-up display projects vehicle information onto the windshield, including speed, gear selection and engine speed. Drivers benefit by not having to take their eyes off the road. Audio features include an AM/FM radio, steering wheel mounted audio controls, and 10 speakers, providing excellent sound throughout the cabin. Mazda also prioritized safety and security with features such as: dual front impact airbags, head curtain airbags, traction control, brake assist, ignition disabling, an emergency communication system, and 4 wheel disc brakes with ABS. Electronic stability control ensures solid grip atop the road surface, no matter how challenging the driving conditions. We pride ourselves in consistently exceeding our customer's expectations. Stop by our dealership or give us a call for more information.


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Windows 8.1, 10 Windows Photo Viewer Updated with Printing Issues Fix
Several Windows users, especially Windows 8 and Windows 8.1 owners, have been reporting printing problems with the Windows Photo Viewer application, especially with XPS drivers. Now, Microsoft has issued an update to fix the problems.
Microsoft's Windows Photo Viewer software is used by millions of users across the world and it was only natural that some issues would have appeared. In the latest Patch Tuesday security bulletin release, Microsoft has made available an update for Windows Photo Viewer that seems to be related to printing issues. Dubbed as:"Windows Photo Viewer prints white lines when you use an XPS driver to print photos in Windows", here's its description:
You install update 2670838 on a computer that is running Windows 7 or Windows Server 2008 R2. Or, you are using a computer that is running Windows RT, Windows 8, Windows Server 2012, Windows RT 8.1, Windows 8.1, or Windows Server 2012 R2. You use Windows Photo Viewer to open a picture that is larger than 500 pixels. For example, the size of the picture is 768*1024. You print the picture by using a printer that uses the XPS driver. In this scenario, there are white lines in the printed picture every 500 pixels.
For those of you who don't know, an XPS file is Microsoft's "less-compatible" version of a PDF file. We are not sure how many are those affected by these problems with XPS drivers when printing from Windows 8.1, Windows 8 or other versions, but it's great an updated has been put in place to take care of the problems. As part of the latest Patch Tuesday, Microsoft has also updated SkyDrive and their Malicious Software Removal Tool.
Update: if you got the 'can't open this picture' error, you can follow up[ with the steps from this fix guide. If you cannot view ANY photos in Windows 10, 8.1 or 8, that might be a system error, so be sure you check this article. For any information about 'how to open' a type of files, we have the right instruction right here, in our dedicated article.
How to replace Photo Viewer in Windows 8, 10
Now, what is important for you to know, is that Photo Viewer is not the only app that can help you open different types of image files. Though it is free, there is much other free software that is a lot better than it. For example, you can check this list of free photo viewers that will surely open your photos.
Editor's Note: This post was originally published in December 2013 and has been since revamped and updated for freshness, accuracy, and comprehensiveness.
Read Also: Epson Printer Memory Card Readers Not Accessible in Windows 8
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The European Cyber Security Conference (organised by Forum Europe) provides a platform for key policymakers and stakeholders to discuss and debate the most pertinent issues affecting the security and safety of the digital space.
On October 25th the IT ACADEMY is dedicating a whole day to the topic of Cyber Security with the fourth edition of CyberSec Day.
The event is gathering cybersecurity experts giving valuable insights on the fast evolving cybersecurity landscape; over the last years companies have been subject to increasingly sophisticated cyber attacks: they have had to evolve their approach to cybersecurity over time and today face the challenge of how to keep it aligned with the business strategy.
The workshop is going to draw attention to the fundamental importance of cybersecurity challenges in manufacturing environments, where they are not yet fully recognised and addressed.
Cybersecurity Week Luxembourg is an advocacy-campaign week, which aims to raise awareness of cybersecurity threats, promote cybersecurity among citizens, corporates and SMEs, and provide up-to-date security information through education and sharing best practices.
Cyberwatching.eu is organizing its first Annual Event on 08 October 2018.
The annual Workshop will be held in Athens and Krakow with three tracks covering key topics in cybersecurity and privacy for different stakeholders.
1 - Aligning and prioritising EU and international Cybersecurity and Privacy - Krakow, Poland 08.10.2018, 11:40-13:30
Cyberwatching.eu is organizing its first Annual Workshop at Cybersec Forum 2018 in Krakow, Poland.
The Annual Workshop will be organized in three sessions :
The next Cyberwatching.eu workshops, at Cybersec Forum in Krakow, will be a forum to better discuss how to achieve greater alignment internationally on cybersecurity and privacy issues.
ENISA and Cyberwatching.eu co-organize in October 8, 2018 a workshop on security measures (article 32 GDPR) in Athens.
Ethical and Legal Aspects of Autonomous Security Systems
An international conference to be held at the University of Zurich in Switzerland on May 2nd-3rd, 2019, aims to explore the ethical and legal aspects of autonomous systems in the security sector. Among others, autonomous systems in cybersecurity are discussed in the conference, that is co-supported by CANVAS.
Philip G. Alston, New York University and UN Special Rapporteur
Extreme Poverty and Human Rights: Artificial Intelligence as a Threat to Human Rights?
Cybertech is the cyber industry's foremost B2B networking platform conducting industry-related events all around the globe, the go-to place to learn all about the latest technological innovations, threats, and solutions to combating threats within the global cyber arena.
Cyberwatching.eu has received funding from the European Union's Horizon 2020 research and innovation programme under grant agreement No 740129. The content of this website does not represent the opinion of the European Commission, and the European Commission is not responsible for any use that might be made of such content. Privacy Policy | Disclaimer / Terms and Conditions of Use


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We are always keen to hear from anyone, aged 16 and over, who would like to get involved, and no prior experience is necessary.
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Where necessary, training is provided for what is a really fun and rewarding pastime, so if you would like to find out what is involved, just get in touch or book a place on our Volunteer Open Days on 7 April or 1 June.
There is no minimum commitment and you are free to attend as often as you wish, but beware… steam railways are addictive!
Call 01208 73555 to book your place. We look forward to seeing you there!
Don't miss this and our other 2019 special events. Follow us on Facebook, Twitter and Instagram, and get on-board with our mailing list for all the latest news, events and offers.


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Being pregnant, wait for a child is a wonderful time, but often puts the veins to the test. The risk of increase of venous insufficiency is stronger from the second pregnancy. During pregnancy, solutions exist to combat heavy legs and venous insufficiency. In, you will know in 9 key stages, all means for the solution of contention that fits you perfectly.
Stockings or pantyhose of contention for fight against venous insufficiency, heavy legs and varicose veins during pregnancy
If you are pregnant, the daily use of tights and low compression (commonly called low contention) is particularly suitable for avoid Frank degradation of your network, especially if you already have a slight failure or a hereditary factor in your family.
Get the mid-low (low shank) that don't offer full protection of your leg, thighs being without compression of your choice. They are practical, that's undeniable, but less effective protection from venous insufficiency.
In contrast, stockings and tights of contention will contain all of your limbs to avoid the dilation of the veins and limit the risk of phlebitis.
The purchase of low or tights of restraint is done after a medical diagnosis clearly is even during pregnancy
Stockings can be purchased after the installation of a diagnosis of a physician (attending or specialist) or a wise woman. It is a medical device that has nothing to do with stockings classic city. Their prescription meets precise diagnosis with the determination of compression including the.
At the level of the class or the strength of stockings, the requirements are often products of class 2 or 3 depending on the diagnosis.
Downs against venous insufficiency for pregnant women
Long choose them (my eBook can help you), the low autofixants are practical to put, but give a sexy connotation to the pregnant woman. This image can create a psychological barrier among the expectant mother, given the event that prepares.
The contention tights specially designed for pregnancy
The tights of contention for pregnant women adapt to the stomach to not tighten the abdominal area. Their port remains comfortable and aesthetically, nothing can distinguish it from a classic down-nylon for an outside eye. All manufacturers of support stockings offer. So there is an important choice. Orthopedic specialists can help you choose.
Buy stockings and pantyhose of contention during pregnancy by going to a specialist in orthopaedics
There is a lot of contention tights suitable for pregnant women. As always, insofar as it is a medical device, and that in addition to buy tights of restraint, it must especially be and so support them, both buy useful to a specialist. A specialized pharmacy or store orthopedics will help you determine your needs with professionalism and rigour by taking the time to try in adapted conditions (specific, taking measures… changing room).
According to the development of pregnancy, it is possible that discomfort is felt in the stomach during the last months. Normally, this is provided by manufacturers by making the sticky to the very stretchy belly. If this is too painful, return take advice to the Orthopedic chemist where you bought the maternity pants.
During pregnancy, putting socks and tights of contention may be facilitated by a low-wear
To put stockings during your pregnancy, you can help with a low-wear of contention. The use of this accessory is very convenient, if you get it right. There are more or less light, more or less easy to use templates.
With thanks to its 9 steps you will have keys, simple and efficient techniques to avoid mistakes and finally to buy items of contention that you really relieve.
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Spain's new royals spend big on airplane food
Segovian suckling pig (Spain's finest) is on the royal plane menu. Photo: Fadel Senna/AFP, Puroticorico/Flickr
25 July 2014
Be honest, who hasn't dreamed of working remotely with all the perks of employment? If you've got the skills, you only need to look UP to make that dream a reality.


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We were privileged to have worked with hundreds of top artists and educators who authored the original magazine articles and then recorded audio lessons in their own studios. While video is the medium of choice today, these 1,200+ audio lessons still deliver amazing instruction from some of the best in the biz — perfect for those long drives and commutes!
Travis Perry's eight year old daughter wanted to quit playing the guitar as well, which is why he decided it is high time that somebody decided to do something about the common guitar "obstacles". Travis Perry states that the area he lives in was hit pretty hard during the economical downfall, which is why it is very important to him to keep the manufacturing and the jobs in the United States of America. Travis Perry also states that it means a lot to him, when he is able to give back to the community.
AGE CAN'T HINDER YOU – Working off of muscle memory and visual assistance, ChordBuddy is designed for players of every age. In fact, ChordBuddy is well-suited for those looking to play guitar with arthritis, offering a pain-free method of playing your favorite song. Utilizing ChordBuddy also allows you to learn the guitar on your own, eliminating the need for long guitar lessons with an instructor, which can result in prolonged joint pain.


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The Aqueous Semi Flush is an Indoor Ceiling fixture by Kalco Lighting. This fixture is recommended for the beautification and illumination of a variety of rooms including but not limited to Bathroom, Hallway, Kitchen, Living Room, Bedroom, etc.
This Aqueous Semi-Flush Mount is a/an Kalco Lighitng design.
The design of our Aqueous Collection was inspired by the ripples of a stone thrown into the ocean. This collection features a slim stem with metal cables, finished in KalcoÕs exclusive Satin Nickel, suspending a bowl of beautiful white frosted Costa Glass. The concentric circles etched into the bowl soften this sleek, modern pendant light.
Prop-65 CA Residents: WARNING: Cancer and Reproductive Harm - www.P65Warnings.ca.gov
- Height -15.5 inches Diameter- 15.38 inches
- Weight - 11 lbs
- Backplate/Canopy Width - 4.69 inches Backplate/Canopy Height - 0.75 inches
- Wire Length - 6 inches
- Lamping - 3 100W 120V E26 Medium
- Bulb Included - No
Listing & Safety Rating Location:
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- Safety Rating Location - Dry
About Kalco Lighitng
Kalco Lighting has been a leader in the Lighting Industry for over 34 years. Kalco Lighting's dedication to Design, Sirvice and Quality is the foundation for their success, and they are confident that in their presentation of hand- crafted and hand finished fixtures and furnishings will continue the tradition. Kalco Lighting currently offers Vanity Fixtures, Flush Mounts, Mini Pendants, Pot Racks, Semi Flush Mounts, Wall Mounts and Post Mounts. The designs and quality of Kalco Lighting fixtures lure the attention of the distinct eye and can be found in magnificent homes and upscale hospitality environments.
While browsing through Kalco Lighting's collections. keep in mind that they offer a variety of finish, glass and shade options. This provides the most unique opportunity for you to create a unique design to complement any decor.
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Moving house is among life's most stressful experiences. It consumes gobs of your time, is constantly more complicated than you anticipate, and risks damage to your precious ownerships. Then there are the unknowns of a brand-new house in a new town. So you do not need unpleasant surprises from a unethical or inexperienced moving business. In truth, you want your moving business to make all of it much easier!
Get The Most Effective Long Distance Mover In Kings Park NY 11754
Two. Corporations will be capable to provide you a quote for your relocation – this represents that you can spending plan ahead of time as to how substantially your move will price tag, and can find out how considerably earnings you have left for other costs.
The finest business for this will be really hectic, so you'll have to arrange your relocation well ahead of time. If you want movers and packers need to be offered on a day that is finest for you, make a deposit to book their services. It takes a great deal of equipment for local shifting companies and for a nationwide shifting company to finish your relocation.
Choose Your Moving Services
Finding a long distance mover requires correct focus on certain aspects. Because you are relocating to New york city it is much better a hire a business which understands that city thoroughly and has correct storage centers there. You might require to avail such centers when you are making an overall relocation.
Have them come over and take an appearance at the items that require to be moved once you have actually chosen on the company you are hiring. It is just after doing so that they will have the ability to give you an estimate of just how much the entire process will cost you. , if you have a spending plan it is much better to try and work within it..
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3 Houston Movers – Houston Movers is the regional branch of a nationwide moving and storage business. They offer regional and long distance moving, in addition to storage for property and business clients.
Begin out by finding the business that provide the services you are looking for when it comes time to discover the moving company you need. Your next step is to gather moving quotes when you find those services. When you employ that specific company, a moving quote is an estimate of how much you will pay. Your objective in moving quotes is to find the most inexpensive moving service that provides what you require in regards to moving.
A much better method to sidetrack your children from unfavorable emotions is to indulge in some creative activity. For instance, you can spend a knowing session with your kids where you can find out a new language specifically the language of the nation where you are preparing to move. If they see that even you are discovering the language along with them, and your children will enjoy the session.


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⚠ Version 1 of The Plant List has been superseded.
This name is in version 1.1 of The Plant List, record kew-2472605, and has not been changed.
This name is a synonym of Zamia pygmaea .
The record derives from WCSP which reports it as a synonym (record
378954) with original publication details: Prodr. 16(2): 543 1868.
Full publication details for this name can be found in IPNI:


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Dr. Frank Greer, from the Committee on Nutrition, American Academy of Pediatrics said, "Infants need cereals to grow and develop all the muscles. They ought to be fed routinely"
The new born baby certainly requires nutritious diet that is effective to every limb of his body. It ought not to be extra neither less in quantity and the proportion of impact. In that case, cereals have a significant role. In most candid tone, baby cereals as the baby food have made a huge swing in the past many years. Earlier being rejected as an essential diet, cereals now have gained foremost priority as an infant diet. Slammed in blogs as toxic and over processed commodity, these get you the relevant place in the list of diets essential for children.
Some imperative reasons which support the cereals as an essential and healthy diet;
Nowadays, the baby cereals are considered more important and give the best in every regard to the toddler. These have become the best choice for the lethargic parents who at some point of time really feel fatigued to feed their baby every type of meal. Organic cereals are the supersonic choice for them. They get your baby the best health and make sure he or she is strong enough for the future. While contemplating about the best health, one may fall flat to locate something exceptional, cereals are the valuable choice.
Healthy baby pounce on baby cereals every day.
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Revolving Rack Revolving Rack Multi Use Pocket Spinner Rack
March 21, 2019 0 By
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4 Comments
- 42
Is this used in the same way as in English for going to a doctor's practice because you're sick, or just in the literal sense of visually percieving a doctor?
October 25, 2016
- 321
This one was tricky at full speed "type what you hear" ("tir", not ti'r), but the slow version is nice.
March 24, 2019


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Canyonwest Cases
Link to Canyonwest Cases has been recently reported as not working and has been temporarily delisted from our categories
Check related resources in Manufacturers/Shipping Cases
Canyonwest Cases
Stock and Custom Shipping, Equipment, Rackmount, Transport, Tool and Flat Screen TV Cases. Waterproof cases and Custom Foam Inserts.
By Don Beauvais (Bovay) Hits: 114 | Votes: 0 | Rating: 0.00
About Canyonwest CasesThe resource is currently listed in dxzone.com in a single category. The main category is Shipping Cases that is about Shipping cases. This link is listed in our web site directory since Sunday Sep 29 2013, and till today "Canyonwest Cases" has been followed for a total of 114 times. So far no one has rated yet, so be the first to rate this link !
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Every Monday, from 04/29/2019 to 08/26/2019, 12:30 PM - 2:00 PM
Ruby Lin, Helena To, Judy Lee
Who's it for:
This 4-month study is for women who works in Central and would like to invest one lunchtime weekly in digging into the Word of God. No prior knowledge is required.
We are surrounded by a world that's watching us, waiting to see if what we say is true--if we really believe what we say and "walk the walk we talk."
That thought may seem overwhelming, even intimidating. But this study by Kay Arthur is ready to guide us into a deeper understanding of God's Word. This study of vital passages from Ephesians will help us discover what God says about the lifestyle of a true believer. And it will equip us to live in a manner worthy of our calling - with the ultimate goal of developing a life marked by maturity, Christ-likeness, and peace.
Discussion, Prayer, Fellowship
For enquiries, please contact .


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My return flight from Bangkok was at 9.45 at the night but the bus from Pattaya dropped me at the Suvarnabhumi airport in Bangkok at 4.45 pm. I had flat five hours to loiter around. The first thing I did was to get my boarding pass. I got it in a jiffy. While going for
Category: Uncategorized
BJP should look beyond Ram, Ayodhya and Cow
The employees were at leisure in Jawahar Bhawan, the building in Lucknow housing over a dozen government departments, when the other day the discussions veered to Congress' performance in three states where results of assembly elections were announced recently. Over a dozen employees were seen animatedly analysing the results of Madhya Pradesh, Rajasthan and Chhattiagarh
Puppies Tryst with Rain
After a long dry spell Lucknow, the city of Nawabs, got the first monsoon shower on Monday – July 30. It did not rain, but poured as if Indra Devta telling Lucknowiites never ever complain about rain (lack of it rather). My this blog is not about rain – but about three street puppies –
Dahakti Jawani, Mahakta Husn
It was a lazy Sunday evening. The attendance in the newsroom was very thin. Our quintessential Bhatt Sahib strolled down the aisle of newsroom where our Sport in-charge sits said something about 'Dahakti Jawani, Mahakta Husn'. I was busy giving final touch to the Prime Minister Narendra Modi's speech which he had delivered during Ground
The New Year Celebration When Cacophony Was Given a Miss
New Year means a big celebration. Bonfire is lit in the compound of my house under mango trees and we (all relatives and friends) collectively cook chicken and other delicacies over earthen oven where food is cooked over wooden fire. The preparation for new year celebration starts early when few branches of Mango trees are


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Waite 'n Sea
$49,900 – 2 Bedroom, 1 and 1/2 Bath – Incredible Ocean View!
This is one cool place! Located in the fabulous, exclusive community of Rancho La Bufadora. Great summertime activities nearby; Kayaking, Diving, Fishing, Hiking; Restaurants and Gift Shops; Beautiful Scenery, Tourist Attractions and more!
Amenities include:
- Large enclosed, wind-proof, courtyard for those big gatherings
- Huge great room with custom wood and stone fireplace
- Beautiful Mexican tile throughout the entire house
- Outside deck overlooking the ocean
Kitchen is unfinished, and 1/2 bath is unfinished. House is as-is.


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Resbond™ Ultra Temp 904 is a smooth paste that is easily applied to ceramics, graphite and metals. Cures to form a reliable adhesive bond, protective coating and encapsulant. Ideal for electronics, semiconductor, instrumentation, aerospace and automotive. read more
1555 Bishop Street, Unit 6 Cambridge, ON N1R 7J4 Tel: 800-828-1004View company website
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"Awesome" update features for Asus Transformer Prime outed; update due March 29th
posted by Alan F. / Mar 28, 2012, 6:00 PM
Other updates include the new UI and greater content for Asus Vibe which is changing from 1.0 to 2.0, the change in the Android Market, Google Books and Google Music to their proper Google Play counterparts, and an update to the camera that will allow a future firmware update to imrove the ol' shooter. After the update, you will be able to hook up your tablet to your television via the HDMI port and view it in landscape or portrait. Finally, you gain the ability to support USB LAN connections by using a USB-to-Ethernet UX cable.
You might not have that long to wait for the update as it is expected to roll out in some regions on Friday.
source: Asus (translated) via Phandroid
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- Display 10.1" 1280 x 800 pixels
- Camera 8 MP / Other front
- Processor NVIDIA Tegra 3, Quad-core, 1300 MHz
- Memory
- Storage 64 GB + microSDHC
- Battery
12 Comments
1. sorcio46
Posts: 435; Member since: Jul 27, 2011
Awesome, waiting for the update :-)
posted on Mar 28, 2012, 6:34 PM 2
9. bobfreking55
Posts: 866; Member since: Jul 15, 2011
DOWNLOADING!!! so excited.
posted on Mar 29, 2012, 6:46 AM 0
11. bobfreking55
Posts: 866; Member since: Jul 15, 2011
wait, nothing happened lol. there's play music, vibe free music, but no face unlock... and stuff
posted on Mar 29, 2012, 7:12 AM 0
Posts: 535; Member since: Mar 28, 2012
Awesome waiting to buy one! With QC A15
posted on Mar 28, 2012, 6:43 PM 0
8. sprockkets
Posts: 1612; Member since: Jan 16, 2012
Guess you are getting a Krait LTE version then.
posted on Mar 28, 2012, 10:44 PM 0
Posts: 535; Member since: Mar 28, 2012
Or the exynos!
posted on Mar 28, 2012, 7:20 PM 0
5. rizzell
Posts: 24; Member since: Dec 31, 2011
Is this tablet still availble. Its nowhere to be found and no one seems to be getting anymore in stock. Even Staples says clearance item.
posted on Mar 28, 2012, 8:33 PM 2
10. TrainFromUkraine
Posts: 95; Member since: Mar 26, 2012
Has Asus fixed GPS and Wi-Fi issues on TP or are they both still weak?
posted on Mar 29, 2012, 7:01 AM 0
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