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Solubility of organic mixtures in water.

The solubilities of several chlorobenzenes and other mixtures in water have been determined. The results varied with the phase of the solute mixture and the hydrophilicity of the components and were interpreted through activity coefficients calculated by the UNIFAC equation. It was found that mixtures of structurally related hydrophobic liquids were near ideal in the organic phase; in the aqueous phase activity coefficient of a component was unaffected by the presence of consolutes. Increasing hydrophilicity of the solutes lead to deviations from ideality in the organic phase, but these could be largely accounted for by the UNIFAC equation. For mixtures of solids which did not interact, the components tended to behave independently of one another, and their solubilities were approximately additive. The behavior of mixtures of liquids and solids was intermediate between that of liquid mixtures and that of mixtures of solids. The application of these results to the toxicity of organic mixtures in water is discussed.