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Exciton-Magnon Transition in Linear Chain Compound CsCoCl3·2H2O

The crystal field absorption spectra in the near infrared to visible regions of CsCoCl 3 ·2H 2 O were investigated. All of the absorption bands were well assiged by taking the crystal field and Racah parameters as D q =720 cm -1 , B =920 cm -1 and C =4320 cm -1 , respectively. In the spin forbidden transition 4 T 1 ( 4 F )→ 2 T 1 ( 2 P ) the exciton line and its magnon sideband were observed. The one-dimensionality of magnetic properties is reflected in the temperature dependence of the peak energy and the integrated intensity of the magnon sideband.