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Two-photon chiro-optical properties of gold Au25 nanoclusters.

Atomically-precise chiral gold nanoclusters hold promise for an accurate manipulation of chiro-optical properties, both in linear and nonlinear optics regimes. Here, we present the determination of two-photon linear-circular dichroism and two-photon circular dichroism (TPCD) of Au25[(Capt)18]- (where Capt is captopril). TPCD is found to be two orders of magnitude higher than one-photon circular dichroism.