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Tracing the sources of the different magnetic behavior in the two phases of the bistable (BDTA)2[Co(mnt)2] compound.

A complete computational study of the magnetic properties of the two known phases of the bistable (BDTA)(2)[Co(mnt)(2)] compound is presented. The origin of their different magnetic properties can be traced to a variation in the values of the g tensor, together with a hitherto unknown change in the J(AB) values and their magnetic topology.