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Energy, Particle and Photon Fluxes in Molecular Junctions.

Electroluminescence from a current-carrying molecular junction at steady-state is simulated. Both (charge) particle and energy conservations are satisfied by a perturbative expansion in the radiation/matter coupling. Our approach makes it possible to adopt standard tools of traditional (equilibrium) spectroscopy to study signals from open-systems such as molecular junctions. The non-perturbative analysis of spontaneous light emission signals coincides with the perturbative approach for weak molecule-field coupling.