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Resolution enhanced photothermal imaging by high-order correlation.

Laser scanning photothermal imaging offers a powerful non-destructive testing tool to visualize subsurface structures of opaque materials, but it suffers the resolution limit imposed by thermal diffusion. To overcome this physical obstacle, a tightly focused excitation beam with a high repetition rate is usually used to improve the spatial resolution. Here, we demonstrate that the resolution of photothermal imaging could be enhanced using the high-order correlation imaging method inspired by correlated optical imaging. By carefully designing the laser scanning and modulation behavior, we can individually control the statistical properties of isolated hotspots induced by lasers. Imaging reconstructions of subsurface structures are performed afterward by reading out time-fluctuated thermal images. Moreover, the resolution can be further enhanced by using the high-order correlation, which enables a new way for highly resolved thermal imaging and metrology applications.