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Measurement of OH density and air–helium mixture ratio in an atmospheric-pressure helium plasma jet

The absolute density of OH radicals in an atmospheric-pressure helium plasma jet is measured using laser-induced fluorescence (LIF). The plasma jet is generated in room air by applying a pulsed high voltage onto a quartz tube with helium gas flow. The time-averaged OH density is 0.10 ppm near the quartz tube nozzle, decreasing away from the nozzle. OH radicals are produced from water vapour in the helium flow, which is humidified by water adsorbed on the inner surface of the helium line and the quartz tube. When helium is artificially humidified using a water bubbler, the OH density increases with humidity and reaches 2.5 ppm when the water vapour content is 200 ppm. Two-dimensional distribution of air–helium mixture ratio in the plasma jet is also measured using the decay rate of the LIF signal waveform which is determined by the quenching rate of laser-excited OH radicals.