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Island Size and Environment Dependence of Adatom Capture: Cu/Co Islands on Ru(0001)

The rate of capture by stable Co islands on Ru(0001) of additionally deposited Cu atoms is quantified using scanning tunneling microscopy, kinetic Monte Carlo simulations, and diffusion equation analyses. We find strong dependence of the capture rates on Co-island size, larger islands showing larger capture rates, qualitatively distinct from self-consistent mean-field predictions. The observed size dependence is shown to reflect larger island-free areas surrounding bigger islands, i.e., a strong correlation between island sizes and separations neglected in mean-field treatments.