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On the control of product yields in the photofragmentation of deuteriumchlorid ions (DCl+).

The prospect of controlling the photofragmentation of deuterium chloride ions (DCl+) via strong ultrashort IR laser pulses has been investigated by a numerical solution of coupled Schrodinger equations. The calculations provide evidence that the ratio of product ion yields Cl+ versus D+ can be manipulated by an appropriate choice of laser pulse parameters, in particular, central laser frequency, pulse duration, intensity, and chirp. The analysis of time-dependent populations reveals competition between intra- and interelectronic state excitations, enabling the understanding of quantum control at the molecular level.