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Solution processed high band‐gap CuInGaS2 thin film for solar cell applications

A high band‐gap (~1.55 eV) chalcopyrite compound film (CuInGaS2) was synthesized by a precursor solution‐based coating method with an oxidation and a sulfurization heat treatment process. The film revealed two distinct morphologies: a densely packed bulk layer and a rough surface layer. We found that the rough surface is attributed to the formation of Ga deficient CuInGaS2 crystallites. Because of the high band‐gap optical property of the CuInGaS2 absorber film, a solar cell device with this film showed a relatively high open circuit voltage (~787 mV) with a power conversion efficiency of 8.28% under standard irradiation conditions. Copyright © 2013 John Wiley & Sons, Ltd.