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Delayed and direct cage exit in photodissociation of Cl2 in solid Ar.

The yield for photodissociation of Cl 2 in solid Ar was measured experimentally as a function of photon energy and studied by molecular dynamics simulations. The results show that separation of the Cl fragments at low energies occurs by delayed exit (t≥3 ps) from the surrounding cage of Ar atoms. Above a photon threshold energy of ≥9.0 eV, there is a switchover to direct cage exit, in which the Cl impulsively knocks a cage atom out of its way