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A fully autonomous ozone, aerosol and nighttime water vapor lidar: a synergistic approach to profiling the atmosphere in the Canadian oil sands region

Abstract. Lidar technology has been rapidly advancing over the past several decades. It
can be used to measure a variety of atmospheric constituents at very high
temporal and spatial resolutions. While the number of lidars continues to
increase worldwide, there is generally a dependency on an operator,
particularly for high-powered lidar systems. Environment and Climate Change
Canada (ECCC) has recently developed a fully autonomous, mobile lidar system
called AMOLITE (Autonomous Mobile Ozone Lidar Instrument for Tropospheric
Experiments) to simultaneously measure the vertical profile of tropospheric
ozone, aerosol and water vapor (nighttime only) from near the ground to
altitudes reaching 10 to 15 km. This current system uses a dual-laser,
dual-lidar design housed in a single climate-controlled trailer. Ozone
profiles are measured by the differential absorption lidar (DIAL) technique
using a single 1 m Raman cell filled with CO2. The DIAL
wavelengths of 287 and 299 nm are generated as the second and third Stokes
lines resulting from stimulated Raman scattering of the cell pumped using the
fourth harmonic of a Nd:YAG laser (266 nm). The aerosol lidar transmits
three wavelengths simultaneously (355, 532 and 1064 nm) employing a detector
designed to measure the three backscatter channels, two nitrogen Raman
channels (387 and 607 nm) and one cross-polarization channel at 355 nm. In
addition, we added a water vapor channel arising from the Raman-shifted
355 nm output (407 nm) to provide nighttime water vapor profiles. AMOLITE
participated in a validation experiment alongside four other ozone DIAL
systems before being deployed to the ECCC Oski-ôtin ground site in the
Alberta oil sands region in November 2016. Ozone was found to increase
throughout the troposphere by as much as a factor of 2 from stratospheric
intrusions. The dry stratospheric air within the intrusion was measured to be
less than 0.2 g kg−1. A biomass burning event that impacted the region
over an 8-day period produced lidar ratios of 35 to 65 sr at 355 nm and 40
to 100 sr at 532. Over the same period the Ångström exponent
decreased from 1.56±0.2 to 1.35±0.2 in the 2–4 km smoke region.
