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Radiation Decomposition of Chlorates

Radiation induced decomposition yields of chloride, hypochlorite and chlorite have been determined in chlorates of barium, calcium and strontium for different y doses. The G-value of the products in anhydrous barium and calcium chlorates are found to be greater than in the corresponding hydrated forms showing that the water of crystallization plays a quenching role in the radiation decomposition of chlorates. The results are explained on the assumption that the excitation energy of the fraction of the metal ions is transferred to the water molecules in the crystal lattice resulting in the excitation or decomposition of the water molecules rather than chlorate ions.