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Theory of laser-induced excitation transfer and atomic association. II. Resonances.

We have extended our previous analysis of diatom laser-induced excitation transfer, illustrated by several examples, to include modifications due to laser-induced resonances. Compact and rigorous final results have been obtained through the use of a projection-operator scheme in combination with the ``symmetric-top'' basis set and a full quantal treatment of the radiation field. The principal limitations on our analysis are a neglect of fine-structure coupling and a simplifying assumption that the ground electronic manifold supports no bound nuclear states. Simple order-of-magnitude estimates of the predicted resonant cross sections also are provided.