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Magnetic frustration induced liquid-like short-range ordering in cubic Mn1.5Cr1.5O4

In this report, we have done a detailed investigation on temperature-dependent neutron diffraction patterns to reveal the existence of short-range magnetic ordering above Neel temperature, which persists at low temperature in cubic spinel Mn1.5Cr1.5O4. The inverse susceptibility curve starts to deviate from the Curie–Weiss law below T′ (∼170 K). The magnetic diffuse scattering around the (111) peak also shows a similar feature, which confirms the development of a short-range magnetic correlation below 170 K. This diffuse scattering shows a maximum at TN, 56 K, and then starts to normalize to the magnetic Bragg peaks below TN but never becomes zero. The magnetic frustration present in the system induces a liquid-like short-range ordering, which co-exists along with the long-range ordering in the ferrimagnetic state.