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Coherent control of Forster energy transfer in nanoparticle molecules: energy nanogates and plasmonic heat pulses

We study how Forster energy transfer from a semiconductor quantum dot to a metallic nanoparticle can be gated using quantum coherence in quantum dots. We show this allows us to use a laser field to open the flow of the energy transfer for a given period of time (on-state) before it is switched off to about zero. Utilizing such an energy gating process it is shown that quantum-dot–metallic-nanoparticle systems (meta-molecules) can act as functional nanoheaters capable of generating heat pulses with temporal widths determined by their environmental and physical parameters. We discuss the physics behind the energy nanogates using molecular states of such meta-molecules and the resonance fluorescence of the quantum dots.