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A mechanism for the downturn in inverse susceptibility in triangle-based frustrated spin systems

A mechanism for the downturn of inverse magnetic susceptibility below an intermediate temperature, recently observed in many experiments, is proposed as an intrinsic feature of lattices with triangle-based frustrated geometries. The temperature at the bending of the inverse susceptibility curve may be related to the features of other thermodynamic properties; the hump of the specific heat and the emergence of a 1/3 plateau in magnetization under a magnetic field. This fact is derived through a Monte Carlo simulation study of the Ising model on triangular and kagome lattices, and the exact calculation for the single and small-sized triangle clusters, on both the Ising and Heisenberg models. These results may indicate the dominance of S(Sz) = 1/2 quantum (classical) trimer formation in the intermediate-energy regime in two-dimensional triangle-based lattices.