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Multilayer Localized Adsorption of Gases on Solid Surfaces: Heats of Immersion of Heterogeneous Solid Surfaces

A previously described theory of multilayer adsorption of lattice gases on solid surfaces (Z. phys. Chemie, Leipzig 265 (1984) 929) is applied to develop equations defining the change of the heat of immersion due to an earlier gaseous precoverage. These equations take into account the interactions between adsorbed molecules and the energetic heterogeneity of real solid surfaces. The theory is next applied to description of experimental data for the immersional system: water-quartz.