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Investigation on the pulse response of a spin-exchange relaxation-free comagnetometer.

We investigate the magnetic pulse response of the optically pumped comagnetometer operated in the spin-exchange relaxation-free (SERF) regime. The pulse response model describing the evolution of the coupled spin ensemble of alkali metal and noble gas during and after the pulse is established for the first time. A three-beam comagnetometer is created with a circularly and two linearly polarized lasers to detect the responses in the three axes of the comagnetometer simultaneously and independently. The results indicate that the response to the small pulse excitation is dominated by the electron spins, while the response to the large pulse excitation and both responses after the pulse excitation consist of a fast and a slow oscillation, which are dominated by the electron spins and nuclear spins, respectively. We also observe novel dynamics of the coupled spin ensemble when the nuclear spins are tipped far away from equilibrium. The theory and method presented here can not only facilitate the investigation on the dynamics of the optically pumped coupled spin ensemble, but also shed light on the application of the pulse modulation technology in the SERF comagnetometer.