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Mechanism and Spindynamics of Photoinduced Electron Transfer Reactions

Photoinduced electron transfer in polar solvents generates exciplexes and radical pairs. The specific reactions of these intermediates have been studied for systems with pyrene as the primarily excited acceptor and various aromatic and aliphatic amines as electron donors by measuring exciplex decay times and by evaluating time-resolved extinction measurements carried out with and without an external magnetic field of 500Gauß. The time-independent rate