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Convergence of Adaptive Compression Methods for Hartree‐Fock‐Like Equations

The adaptively compressed exchange (ACE) method provides an efficient way to solve Hartree‐Fock‐like equations in quantum physics, chemistry, and materials science. The key step of the ACE method is to adaptively compress an operator that is possibly dense and full‐rank. In this paper, we present a detailed study of the adaptive compression operation and establish rigorous convergence properties of the adaptive compression method in the context of solving linear eigenvalue problems. Our analysis also elucidates the potential use of the adaptive compression method in a wide range of problems. © 2018 Wiley Periodicals, Inc.