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RELAXATION PROCESS INDUCED BY CORE-SHELL MORPHOLOGY

In this work a new relaxation process due to core-shell morphology of ternary blends was identified. The relaxation spectra of poly(methyl metacrylate) PMMA, polypropylene (PP), polystyrene (PS) ternary blends, that presented a core-shell morphology inferred from linear viscoelastic measurements, presented three relaxation times, one corresponding to the superposition of the relaxation times of the dispersed and matrix phase, a second one corresponding to the relaxation of the shape of the dispersed phase and a fourth long one due to the presence of a core of PS at the interface between PMMA and PP. To the authors' knowledge this relaxation process due to core-shell morphology has never been reported previously.