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The 1-Dimensional Glassy Behavior of Ultraconfined Water Strings.

Water is renowned for its anomalous behaviors, which can be linked to a distributed H-bond network in bulk water. Ul-tra-confinement of the water molecule can remove H-bonding, leaving only molecular water. In natural cordierite crystals, water is trapped in an orthorhombic channel with an average diameter of 5.7 Å, running through the center of the unit cell. Calorimetric measurements reveal the existence of a 1-D glass linked to this water. In these channels, water molecules in truncated, sparse 1-D strings only interact via dipole-dipole correlation. A physical 1-D glass is formed from these strings. This unusual state can be explained by a modified Ising model. This model predicts a dependence of the glass transition temperature, Tg, on the size of these domains. This is confirmed experimentally.