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Polyvariant aggregation in single fluids: thermodynamics and effects on dielectric properties

The theory of chain-like polyvariant association in single fluids is reviewed. The successive derivation of the most common expressions for calculating Kirkwood's correlation factor gd , which is connected with static dielectric permittivity εs , is given. The general theory of polyvariant linear aggregation in monohydric alcohols is presented for the first time. Correlation between adjacent bond states is introduced as a quantitative character r for exhaustive description of supramolecular structure of monohydric alcohols. The influence of isomerism of topologically linear associates on the dipole correlation factor gd has been investigated.