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Lyapunov instability of rigid diatomic molecules in three dimensions.

We study the Lyapunov instability of a three-dimensional fluid composed of rigid diatomic molecules by molecular dynamics simulation. We use center-of-mass coordinates and angular variables for the configurational space variables. The spectra of Lyapunov exponents are obtained for 32 rigid diatomic molecules interacting through the Weeks-Chandler-Andersen potential for various bond lengths and densities. We show the general trends and characteristic features of the spectra of the Lyapunov exponents, and discuss the different contributions between translational and rotational degrees of freedom depending on the density and the bond length from the calculation of the projection of a certain subspace of the tangent space vectors.