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Effects of Ionizing Radiations on the Amount and the Chemical Forms of Tritium Sorbed on the Surface of Borosilicate Glass

The amount and chemical forms of tritium sorbed pn a borosilicate glass were studied by exposing a specimen with gaseous tritium to a 6 Co source. Two patterns were observed: the amount of tritium sorbed on the surface increased with the gamma ray dose absorbed, and the chemical forms of tritium desorbed from the inner layer were completely altered. Similar results were obtained using sorbing tritium gases of different specific activities. From these facts, it was concluded that the chemisorption of tritium was governed by the reaction of long-lived defects formed by radiations with molecular tritium (DT, T2 , etc.). The radiation-induced exchange reaction may also play an important role in the chemisorption.