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Directed assembly of nano-scale phase variants in highly strained BiFeO3 thin films

The delicate balance between elastic energy and electrostatic energy in highly strained BiFeO3 (BFO) thin films results in complex mixed-phase patterns, which poses significant challenges for theoretical understanding and complicates the realization of its full potential in magnetoelectric, electromechanical, and photovoltaic devices. In this letter, we explore in-plane electric field induced phase transition in strain engineered BFO thin films and elucidate the mechanism behind the assembly behavior of complex nano-scale phase domains. Our approach enables deterministic control of phase variants with well-defined structures and orientation, paving the way for designing novel data storage devices based on mixed phase BFO.