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Two-dimensional N-doped Pd/carbon for highly efficient heterogeneous catalysis.

A novel two-dimensional ZIF-derived Pd@CN material prepared via one-step calcination exhibits outstanding catalytic activity in heterogeneous hydrogenation. Its well-developed porous structure, low dimensions and low density make active sites more accessible. This facile and effective strategy can guide the synthesis of highly active and durable Pd@CN catalysts with specific morphologies.