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Synthesis, CO2 Adsorption Performance of Modified MIL-101 with Multi-Wall Carbon Nanotubes

Nearly 40% of the world gas reservoir contains high level of CO2 that stance problems to development. The discovery of natural gas field with CO2 content of as high as 87% in Malaysia poses new challenges in terms of the CO2 separation processes. This research work investigates the potential of MIL(Materials Institute Lavoisier)-101 as CO2 capture and storage candidate by conducting an experiment with different pressure between the synthesised and modified MIL-101 using Multi-wall carbon nano tubes (MWCNTs). To investigate the effect of the MWCNTs in MIL-101 towards CO2 adsorption performance. The synthesized MOFs were characterized using scanning electron microscopy (SEM) for surface morphology, Thermogravimetric analysis (TGA) for thermal stability, X-ray diffraction (XRD) for crystals plane, Brunauer-Emmet-Teller (BET) for surface area and CO2 adsorption performance. The result had showed that the modified MIL-101 enhanced the CO2 adsorption compared to the pure MIL-101. MWCNT@MIL-101 showed the adsorption of CO2 uptake is 0.0029mmole-1/g at 100kPa.