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Quantum transport in CVD graphene synthesized with liquid carbon precursor

Large-area high-quality graphene enabled by chemical vapor deposition (CVD) can possibly pave the path for advanced flexible electronics and spintronics. CVD-grown method utilizing liquid carbon precursor has recently been demonstrated as an appealing choice for mass graphene production, thanks to its low cost and safe operation. However, the quality of the graphene film has been the major obstacle for the implementation of the liquid-precursor-based CVD method. Here we report the growth of centimeter-scale easily-transferable single-layer graphene (SLG) using acetone as a liquid carbon precursor. The dry-transfer technique was used to prepare the graphene device. The typical mobility of the dry-transferred SLG device is as high as 12 500 cm2 V−1 s−1 at room temperature. Thanks to the high quality of the device, the robust quantum Hall effect can survive up to room temperature. The excellent device quality also enables us to observe the Shubnikov–de Haas oscillation in the low magnetic field regime and systemically study the leading scattering mechanism. We extracted both the transport scattering time τ t and the quantum scattering time τ q over a wide range of carrier density. The ratio of the scattering times suggests that the charged-impurity resided near the surface of the graphene restricted the device performance.