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Magnetic Susceptibilities of Transition Metal Solutes in Liquid Se–Te Alloys

The magnetic susceptibilities of 3d-transition metal solutes in liquid Se-Te alloys have been measured in order to study the s-d interaction between the localized d-states and the conduction electrons. The additional susceptibilities of transition metal solutes except V increase monotonically with increasing Se concentration. However, that of V changes with minimum at 40 at% Se. The nonmagnetic states of V, Co and Ni solutes have been discussed with Anderson model. According to this analysis, the changing trend of additional susceptibilities as a function of Se concentration is explained from the decreasing effect of N d and the increasing effect of ( U +4 J )/ Δ .