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The interrelation of magnetic and dielectric properties of CoxMn1 − xS solid solutions

Magnetization of the cation-substituted CoxMn1 − xS sulfides upon cooling in zero and 100 Oe magnetic fields at the temperatures 4–300 K has been measured. Permittivity of these materials at frequencies from 1 to 100 kHz in magnetic and dc electric fields in the 100–300 K temperature range has been determined. Change in the dielectric permittivity under an external magnetic field is found to have a maximum in the temperature ranges of T1 ∼ (110–120 K) and T2 ∼ (230–250 K). Formation of spontaneous magnetic moment and the rise of magnetic susceptibility are revealed at the same temperatures in the CoxMn1 − xS solid solutions. Features of the magnetoelectric properties of the sulfides have been explained by orbital ordering.