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Collective Relaxation, Single Particle Motion and Short Range Order in α′-NbDx: A Quasielastic Neutron Scattering Study

Applying both incoherent and coherent quasielastic neutron scattering we have studied simultaneously single particle motion, collective relaxation and short range order of deuterium in a'-NbD*. A comparison with recent Monte Carlo simulations leads to a consistent description of all results in terms of strongly repulsive deuterium —deuterium interactions. Relating the independently determined tracer and chemical diffusion coefficients with the also measured structure factor we show experimentally that for lattice gases the de Gennes narrowing ansatz needs to be modified by correlation factors.