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Some quantitative aspects of ionic melt microstructure

Computer generated configurations of molten KCl are used to elucidate some aspects of the equilibrium microstructure of ionic liquids. Information obtained by analysis of the previously reported pair distribution functions is expanded by considering corresponding fluctuation functions. The role of Coulombic forces in ionic melts is further illuminated by comparing the indiscriminate distributions of ions with those obtained for atoms in liquid argon. The V -T dependence of structure and ionic radius ratio effects are briefly considered. Current theoretical models are not conformal with the computed microstructure.