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Synthesis and Electronic Behavior of a Ternary, Alternating Zirconium‐Phenylene‐Tin Hybrid Copolymer

A ternary, networked zirconium‐phenylene‐tin hybrid copolymer was synthesized by initially reacting zirconium n‐butoxide with 4‐hydroxythiophenol followed by a reaction with tin t‐butoxide, and its electronic behavior was examined by UV‐VIS and ESR spectral analyses and ab‐initio calculation of copolymer models. It was shown that an electron transfer takes place initially from the phenylene moiety to LUMO of tin atom followed by the second electron transfer to LUMO+1 of zirconium atom.