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"Supramolecular" Solid-State Chemistry: Interpenetrating Diamond-Type Frameworks of U4+ Ions Linked by S,S'-Bidentate P2 S62- Molecular Rods in UP4 S12.

Inseparably interwoven are three independent polymeric diamond-type U(P2 S6 )2 frameworks in the structure of the title compound. The linear P2 S6 units act as molecular rods linking the pseudotetrahedral U4+ centers. U(P2 S6 )2 may be viewed as a coordination polymer which is formed from U/P/S melts by the solid-state equivalent of the self-assembly reactions in solution.