Quantum theory of light and noise polarization in nonlinear optics
  We present a consistent quantum theory of the electromagnetic field in nonlinearly responding causal media, with special emphasis on $\chi^{(2)}$ media. Starting from QED in linearly responding causal media, we develop a method to construct the nonlinear Hamiltonian expressed in terms of the complex nonlinear susceptibility in a quantum mechanically consistent way. In particular we show that the method yields the nonlinear noise polarization, which together with the linear one is responsible for intrinsic quantum decoherence. 
Stefan Scheel and Dirk-Gunnar Welsch